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manuscript_SPL_final.pdf (23.26 MB)

Defect Engineering for Quantum Grade Rare-Earth Nanocrystals

preprint
submitted on 08.05.2020, 15:43 and posted on 12.05.2020, 04:52 by Shuping Liu, Alexandre Fossati, Diana Serrano, Alexandre Tallaire, Alban Ferrier, Philippe Goldner

In this work, we demonstrate that a novel post-treatment process that includes multi-step high-temperature annealing followed by high-power microwave oxygen plasma processing advantageously improves key properties for quantum technologies. We obtain single crystalline nanoparticles (NPs) of 100 nm diameter, presenting bulk-like inhomogeneous linewidths and population lifetimes (T1). Furthermore, a significant coherence lifetime (T2) extension, up to a factor of 5, is successfully achieved by modifying the oxygen-related point defects in the

NPs by the oxygen plasma treatment. These promising results confirm the potential of these engineered RE NPs to integrate devices such as cavity-based single photon sources, quantum memories and processors. In addition, our strategy could be applied to a large variety of oxides to obtain outstanding crystalline quality NPs for a broad range of applications.


Funding

NanOQTech project

History

Email Address of Submitting Author

diana.serrano@chimieparistech.psl.eu

Institution

Institut de Recherche de Chimie Paris - Chimie Paristech

Country

France

ORCID For Submitting Author

0000-0002-9478-3776

Declaration of Conflict of Interest

None

Version Notes

author version

Exports