The Sensitivity of Cu for Electrochemical Carbon Dioxide Reduction to Hydrocarbons as Revealed by High Throughput Experiments

Yunchieh Lai; Ryan J. R. Jones; Yu Wang; Lan Zhou; Matthias Richter; John Gregoire

doi:10.26434/chemrxiv.9961718.v1

Catalysis

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The Sensitivity of Cu for Electrochemical Carbon Dioxide Reduction to Hydrocarbons as Revealed by High Throughput Experiments

15 October 2019, Version 1

Working Paper

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This content is a preprint and has not undergone peer review at the time of posting.

Abstract

Electrochemical CO2 reduction to valuable products is a centerpiece of future energy technologies that relies on identificaiton of new catalysts. We present accelerated screening of Cu bimetallic alloys, revealing remarkable sensitivity to alloy concentration that indicates the segregation of alloying elements to critical sites for hydrocarbon formation.

Keywords

Carbon Dioxide Reduction Electrocatalysts Electrochemical conversion

High Throughput Screening

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